We use satellite observations of atmospheric methane from the TROPOMI instrument to estimate total annual methane emissions for 2019–2023 from four large Southeast US landfills with gas collection and control systems. The emissions are on average 6× higher than the values reported by the landfills to the US Greenhouse Gas Reporting Program (GHGRP) which are used by the US Environmental Protection Agency for its national Greenhouse Gas Inventory (GHGI). We find increasing emissions over the 2019–2023 period whereas the GHGRP reports a decrease. The GHGRP requires gas-collecting landfills to estimate their annual emissions either with a recovery-first model (estimating emissions as a function of methane recovered) or a generation-first model (estimating emissions from a first-order decay applied to waste-in-place). All four landfills choose to use the recovery-first model, which yields emissions that are one-quarter of those from the generation-first model and decreasing over 2019–2023, in contrast with the TROPOMI observations. Our TROPOMI estimates for two of the landfills agree with the generation-first model, with increasing emissions over 2019–2023 due to increasing waste-in-place or decreasing methane recovery, and are still higher than the generation-first model for the other two landfills. Further examination of the GHGRP emissions from all reporting landfills in the US shows that the 19% decrease in landfill emissions reported by the GHGI over 2005–2022 reflects an increasing preference for the recovery-first model by the reporting landfills, rather than an actual emission decrease. The generation-first model would imply an increase in landfill emissions over 2013–2022, and this is more consistent with atmospheric observations.
We use satellite observations of carbon monoxide (CO) to estimate CO emissions from European integrated iron and steel plants, the continent’s highest-emitting CO point sources. We perform analytical inversions to estimate emissions from 21 individual plants using observations from the TROPOspheric Monitoring Instrument (TROPOMI) for 2019. As prior emissions, we use values reported by the facilities to the European Pollutant Release and Transfer Register (E-PRTR). These reported emissions vary in estimation methodology, including both measurements and calculations. With the Weather Research and Forecasting (WRF) model, we perform an ensemble of simulations with different transport settings to best replicate the observed emission plumes for each day and site. Comparing the inversion-based emission estimates to the E-PRTR reports, nine of the plants agree within uncertainties. For the remaining plants, we generally find lower emission rates than reported. Our posterior emission estimates are well constrained by the satellite observations (90 % of the plants have averaging kernel sensitivities above 0.7) except for a few low-emitting or coastal sites. We find agreement between our inversion results and emissions we estimate using the cross-sectional flux (CSF) method for the seven most strongly emitting plants, building further confidence in the inversion estimates. Finally, for four plants with large year-to-year variability in reported emission rates or large differences between the reported emission rate and our posterior estimate, we extend our analysis to 2020. We find no evidence in either the observed carbon monoxide concentrations or our inversion results for strong changes in emission rates. This demonstrates how satellites can be used to identify potential uncertainties in reported emissions.
Monitoring methane (CH4) emissions from terrestrial ecosystems is essential for assessing the relative contributions of natural and anthropogenic factors leading to climate change and shaping global climate goals. Fires are a significant source of atmospheric CH4, with the increasing frequency of megafires amplifying their impact. Global fire emissions exhibit large spatiotemporal variations, making the magnitude and dynamics difficult to characterize accurately. In this study, we reconstruct global fire CH4 emissions by integrating satellite carbon monoxide (CO)-based atmospheric inversion with well-constrained fire CH4 to CO emission ratio maps. Here we show that global fire CH4 emissions averaged 24.0 (17.7–30.4) Tg yr‑1 from 2003 to 2020, approximately 27% higher (equivalent to 5.1 Tg yr‑1) than average estimates from four widely used fire emission models. This discrepancy likely stems from undetected small fires and underrepresented emission intensities in coarse-resolution data. Our study highlights the value of atmospheric inversion based on fire tracers like CO to track fire-carbon-climate feedback.
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